Aerosols

India's climate research agenda: 2030 and beyond

The Intergovernmental Panel on Climate Change (IPCC), Assessment Report 6 (AR6), stated that the recent climate change is “widespread, rapid, intensifying and unprecedented in thousands of years.” It is further noted: “Climate change is already affecting every region on Earth in multiple ways. The changes we experience will increase with …

Developing and diagnosing climate change indicators of regional aerosol optical properties

Given the importance of aerosol particles to radiative transfer via aerosol-radiation interactions, a methodology for tracking and diagnosing causes of temporal changes in regional-scale aerosol populations is illustrated. The aerosol optical properties tracked include estimates of total columnar burden (aerosol optical depth, AOD), dominant size mode (Ångström exponent, AE), and …

A pan-tropical cascade of fire driven by El Niño/Southern Oscillation

The El Niño/Southern Oscillation (ENSO) has a pronounced influence on year-to-year variations in climate1. The response of fires to this forcing2 is complex and has not been evaluated systematically across different continents. Here we use satellite data to create a climatology of burned-area and fire-emissions responses, drawing on six El …

Complex three-dimensional self-assembly in proxies for atmospheric aerosols

Aerosols are significant to the Earth’s climate, with nearly all atmospheric aerosols containing organic compounds that often contain both hydrophilic and hydrophobic parts. However, the nature of how these compounds are arranged within an aerosol droplet remains unknown. Here we demonstrate that fatty acids in proxies for atmospheric aerosols self-assemble …

Declining pre-monsoon dust loading over South Asia: Signature of a changing regional climate

Desert dust over the Indian region during pre-monsoon season is known to strengthen monsoon circulation, by modulating rainfall through the elevated heat pump (EHP) mechanism. In this context, an insight into long term trends of dust loading over this region is of signifcant importance in understanding monsoon variability. In this …

Aerosol emissions factors from traditional biomass cookstoves in India: insights from field measurements

Residential solid biomass cookstoves are important sources of aerosol emissions in India. Cookstove emissions rates are largely based on laboratory experiments conducted using the standard water-boiling test, but real-world emissions are often higher owing to different stove designs, fuels, and cooking methods. Constraining mass emissions factors (EFs) for prevalent cookstoves …

Indoor human exposure to size-fractionated aerosols during the 2015 Southeast Asian smoke haze and assessment of exposure mitigation strategies

The 2015 smoke haze episode was one of the most severe and prolonged transboundary air pollution events ever seen in Southeast Asia (SEA), affecting the air quality of several countries within the region including Indonesia, Malaysia and Singapore. The 24 h mean outdoor PM2.5 (particulate matter (PM) with aerodynamic diameter …

Data integration model for air quality: a hierarchical approach to the global estimation of exposures to ambient air pollution

Air pollution is a major risk factor for global health, with 3 million deaths annually being attributed to fine particulate matter ambient pollution (PM2.5). The primary source of information for estimating population exposures to air pollution has been measurements from ground monitoring networks but, although coverage is increasing, regions remain …

Dominant control of agriculture and irrigation on urban heat island in India

As is true in many regions, India experiences surface Urban Heat Island (UHI) effect that is well understood, but the causes of the more recently discovered Urban Cool Island (UCI) effect remain poorly constrained. This raises questions about our fundamental understanding of the drivers of rural-urban environmental gradients and hinders …

Fine particle mass, number, surface, area concentration metrics and their correlation in outdoor environments

Exposure to fine particles is measured using metrics such as mass concentration (MC), number concentration (NC) and surface area concentration (SAC). This study aims to find correlation between the three metrics in outdoor environments of a city – city periphery, city centre and on-road. Simultaneous real-time mass, number and surface …

Are the impacts of land use on warming underestimated in climate policy?

While carbon dioxide emissions from energy use must be the primary target of climate change mitigation efforts, land use and land cover change (LULCC) also represent an important source of climate forcing. In this study we compute time series of global surface temperature change separately for LULCC and non-LULCC sources …

Influence of super-parameterization and a higher-order turbulence closure on rainfall bias over Amazonia in Community Atmosphere Model version 5 (CAM5)

We evaluate the Community Atmosphere Model Version 5 (CAM5) with a higher-order turbulence closure scheme, named Cloud Layers Unified By Binomials (CLUBB), and a Multiscale Modeling Framework, referred as the “super-parameterization” (SP) with two different microphysics configurations to investigate their influences on rainfall simulations over Southern Amazonia. The two different …

Using radiocarbon to constrain black and organic carbon aerosol sources in Salt Lake City

Black carbon (BC) and organic carbon (OC) aerosols are important components of fine particulate matter (PM2.5) in polluted urban environments. Quantifying the contribution of fossil fuel and biomass combustion to BC and OC concentrations is critical for developing and validating effective air quality control measures and climate change mitigation policy. …

Aerosols from biomass combustion

The use of biomass for heat and power production is supported in many IEA countries since biomass as a renewable fuel can effectively substitute fossil fuels and consequently reduce fossil CO2. During biomass combustion, inhalable particulate matter smaller than 10 micrometres (PM10) can be generated which can cause adverse health …

Multimodel precipitation responses to removal of U.S. sulfur dioxide emissions

Emissions of aerosols and their precursors are declining due to policies enacted to protect human health, yet we currently lack a full understanding of the magnitude, spatiotemporal pattern, statistical significance, and physical mechanisms of precipitation responses to aerosol reductions. We quantify the global and regional precipitation responses to U.S. SO2 …

Benzene formation in electronic cigarettes

The heating of the fluids used in electronic cigarettes (“e-cigarettes”) used to create “vaping” aerosols is capable of causing a wide range of degradation reaction products. We investigated formation of benzene (an important human carcinogen) from e-cigarette fluids containing propylene glycol (PG), glycerol (GL), benzoic acid, the flavor chemical benzaldehyde, …

Winter fog experiment over the Indo-Gangetic plains of India

The objectives of the Winter Fog Experiment (WIFEX) over the Indo-Gangetic Plains of India are to develop better now-casting and forecasting of winter fog on various time- and spatial scales. Maximum fog occurrence over northwest India is about 48 days (visibility <1000 m) per year, and it occurs mostly during …

Observations of aerosol optical properties at a coastal site in Hong Kong, South China

Temporal variations in aerosol optical properties were investigated at a coastal station in Hong Kong based on the field observation from February 2012 to February 2015. At 550 nm, the average light-scattering (151 ± 100 Mm−1) and absorption coefficients (8.3 ± 6.1 Mm−1) were lower than most of other rural …

Increased atmospheric ammonia over the world’smajor agricultural areas detected from space

This study provides evidence of substantial increases in atmospheric ammonia (NH3) concentrations (14 year) over several of the worlds major agricultural regions, using recently available retrievals from the Atmospheric Infrared Sounder (AIRS) aboard NASA’s Aqua satellite. The main sources of atmospheric NH3 are farming and animal husbandry involving reactive nitrogen …

Decadal-scale relationship between measurements of aerosols, land-use change, and fire over Southeast Asia

A simultaneous analysis of 13 years of remotely sensed data of land cover, fires, precipitation, and aerosols from the MODIS, TRMM, and MISR satellites and the AERONET network over Southeast Asia is performed, leading to a set of robust relationships between land-use change and fire being found on inter-annual and …

Climate engineering by mimicking natural dust climate control: the iron salt aerosol method

Power stations, ships and air traffic are among the most potent greenhouse gas emitters and are primarily responsible for global warming. Iron salt aerosols (ISAs), composed partly of iron and chloride, exert a cooling effect on climate in several ways. This article aims firstly to examine all direct and indirect …

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